A: No. Benchmarks show identical read speeds. The PS2 USB bus is the bottleneck, not the file system. In some cases, exFAT is faster because it doesn't have to manage 4GB clip boundaries.
While it cannot fix the inherently slow USB 1.1 speed of the PS2, it removes the software bottlenecks that made loading painful.
A: Yes, via POPStarter (PS1 emulator for PS2). Place your VCD files in the POPS folder. exFAT finally allows large PS1 multidisc games to be stored as single files.

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